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Silver(I)-catalyzed addition of zirconocenes to epoxy esters: A new entry to 1,4-dicarbonyl compounds and pyridazinones

Wipf, P and Methot, JL (1999) Silver(I)-catalyzed addition of zirconocenes to epoxy esters: A new entry to 1,4-dicarbonyl compounds and pyridazinones. Organic Letters, 1 (8). 1253 - 1255. ISSN 1523-7060

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Abstract

(matrix presented) The Ag(I)-catalyzed tandem epoxy ester rearrangement-dioxycarbenium ion addition reaction with alkenyl zirconocenes provides 1,4-keto esters that can be further converted to substituted pyridazinones. The use of a fluorous tag in a cyclization-assisted cleavage strategy demonstrates the feasibility of extending this methodology to high-throughput organic synthesis.


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Details

Item Type: Article
Status: Published
Creators/Authors:
CreatorsEmailPitt UsernameORCID
Wipf, Ppwipf@pitt.eduPWIPF
Methot, JL
Date: 21 October 1999
Date Type: Publication
Journal or Publication Title: Organic Letters
Volume: 1
Number: 8
Page Range: 1253 - 1255
DOI or Unique Handle: 10.1021/ol990924v
Schools and Programs: Dietrich School of Arts and Sciences > Chemistry
Refereed: Yes
ISSN: 1523-7060
Date Deposited: 22 Jul 2015 14:25
Last Modified: 02 Feb 2019 15:57
URI: http://d-scholarship.pitt.edu/id/eprint/25373

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