ETD

Time-resolved two-photon absorption in quantum dots and polaritons

Public Deposited
Analytics

152 pages

Title
  • Time-resolved two-photon absorption in quantum dots and polaritons
Date modified
  • 08/20/2025
Creator
Abstract
  • We used two-photon absorption to study semiconductor samples. The energy of the photons used to excite the particle is half the energy of the electronic transition. In one set of experiments we have performed time-resolved measurements of the time scale for conversion of excitons in dark states to bright (light-emitting) states in GaAs quantum dots. The dark states are pumped using two-photon absorption, while the bright state emission is observed in single-photon emission. This conversion time is connected to the spin flip time for carriers in the quantum dots. The time scale is found to be of the order of several hundred picoseconds. In a second set of experiments, we performed time-resolved measurements of two-photon excitation directly into microcavity polariton states. Although this process is forbidden by symmetry for light at normal incidence, we observed that it is allowed at non-zero angle of incidence due to state mixing. Fermi's golden rule for bosons states that absorption into a final state is enhanced by the occupation of that state. This thesis reports experiments aimed at using a laser beam to create a condensate and modulate the two-photon absorption of a second beam.
Administrative Note
Date created
Identifier
Keyword
Language
Resource type
Degree discipline
  • Physics
Degree grantor
  • University of Pittsburgh
Degree level
  • Doctoral
Degree name
  • Doctor of Philosophy
Rights statement

MLA citation style (9th ed.)

Gautham, Chitra. Time-resolved Two-photon Absorption In Quantum Dots and Polaritons. . 2016. d-scholarship.pitt.edu/concern/etds/40d5b36e-3260-4a06-a13d-84f1cba780bc.

APA citation style (7th ed.)

G. Chitra. (2016). Time-resolved two-photon absorption in quantum dots and polaritons. https://d-scholarship.pitt.edu/concern/etds/40d5b36e-3260-4a06-a13d-84f1cba780bc

Chicago citation style (CMOS 17, author-date)

Gautham, Chitra. Time-Resolved Two-Photon Absorption In Quantum Dots and Polaritons. 2016. https://d-scholarship.pitt.edu/concern/etds/40d5b36e-3260-4a06-a13d-84f1cba780bc.

Note: These citations are programmatically generated and may be incomplete.

In Collection:
Thumbnail Title Date Uploaded Visibility Actions
26693_Chitra_Gautham_thesis.pdf 26693_Chitra_Gautham_thesis.pdf 2025-08-20 Public Download